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We present the results of a molecular survey of long period comets C/2021 A1 (Leonard) and C/2022 E3 (ZTF). Comet C/2021 A1 was observed with the Institut de radioastronomie millimétrique (IRAM) 30-m radio telescope in November-December 2021 before perihelion (heliocentric distance 1.22 to 0.76 au) when it was closest to the Earth (≈0.24 au). We observed C/2022 E3 in January-February 2023 with theOdin1-m space telescope and IRAM 30-m, shortly after its perihelion at 1.11 au from the Sun, and when it was closest to the Earth (≈0.30 au). Snapshots were obtained during 12–16 November 2021 period for comet C/2021 A1. Spectral surveys were undertaken over the 8–13 December 2021 period for comet C/2021 A1 (8 GHz bandwidth at 3 mm, 16 GHz at 2 mm, and 61 GHz in the 1 mm window) and over the 3–7 February 2023 period for comet C/2022 E3 (25 GHz at 2 mm and 61 GHz at 1 mm). We report detections of 14 molecular species (HCN, HNC, CH₃CN, HNCO, NH₂CHO, CH₃OH, H₂CO, HCOOH, CH₃CHO, H₂S, CS, OCS, C₂H₅OH and aGg’-(CH₂OH)₂) in both comets. In addition, HC₃N, and CH₂OHCHO were marginally detected in C/2021 A1, and CO and H₂O (withOdin) were detected in C/2022 E3. The spatial distribution of several species (HCN, HNC, CS, H₂CO, HNCO, HCOOH, NH₂CHO, and CH₃CHO) is investigated. Significant upper limits on the abundances of other molecules and isotopic ratios are also presented. The activity of comet C/2021 A1 did not vary significantly between 13 November and 13 December 2021, when observations stopped, just before it started to exhibit major outbursts seen in the visible and from observations of the OH radical. Short-term variability in the outgassing of comet C/2022 E3 of the order of ±20% is present and possibly linked to its 8h rotation period. Both comets exhibit rather low abundances relative to water for volatile species such as CO (<2%) and H₂S (0.15%). Methanol is also rather depleted in comet C/2021 A1 (0.9%). Following their revised photo-destruction rates, HNCO and HCOOH abundances in comets observed at millimetre wavelengths have been reevaluated. Both molecules are relatively enriched in these two comets (~0.2% relative to water). Since the combined abundance of these two acids (0.1–1%) is close to that of ammonia in comets, we cannot exclude that these species could be produced by the dissociation of ammonium formate and ammonium cyanate if present in comets. 

We present the results of millimetre-wave spectroscopic observations and spectral surveys of the following short-period comets: 21P/Giacobini-Zinner in September 2018, 41P/Tuttle-Giacobini-Kresák in April 2017, and 64P/Swift-Gehrels and 38P/Stephan-Oterma in December 2018, carried out with the Institut de RadioAstronomie Millimétrique (IRAM) 30-m radio telescope at wavelengths between 1 and 3 mm. Comet 21P was also observed in November 1998 with the IRAM 30-m, James Clerk Maxwell Telescope, and the Caltech submillimeter Observatory radio telescopes at wavelengths from 0.8 to 3 mm. The abundances of the following molecules have been determined in those comets: HCN, CH 3 OH, CS, H 2 CO, CH 3 CN, and H 2 S in comet 21P; HCN and CH 3 OH in 41P; HCN, CH 3 OH, and CS in 64P; and CH 3 OH in 38P. The last three comets, classified as carbon-chain typical from visible spectro-photometry, are relatively rich in methanol (3.5–5% relative to water). On the other hand, comet 21P, classified as carbon-chain depleted, shows abundances relative to water which are low for methanol (1.7%), very low for H 2 S (0.1%), and also relatively low for H 2 CO (0.16%) and CO (<2.5%). Observations of comet 21P do not show any change in activity and composition between the 1998 and 2018 perihelions. Sensitive upper limits on the abundances of other molecules such as CO, HNCO, HNC, or SO are also reported for these comets.